Prep the chicken: Pat the chicken dry and season both sides with salt and pepper. This helps lock in flavor and improves browning if you choose to sear.
Make the seasoning mixture: In a small bowl, combine olive oil, lemon zest and juice, minced garlic, red wine vinegar, oregano, thyme, smoked paprika, and a pinch of salt and pepper.
Stir well.
Layer the base: Add the sliced red onion to the bottom of the slow cooker. Pour in the chicken broth and add the bay leaf.
Optional sear: For extra flavor, quickly sear the chicken in a hot skillet with a little oil, 1–2 minutes per side, just until lightly golden. Not required, but it adds depth.
Add the chicken: Place the chicken on top of the onions.
Pour the seasoning mixture over the chicken, coating it evenly.
Cook low and slow: Cover and cook on Low for 4–5 hours or on High for 2–3 hours, until the chicken is tender and reaches 165°F.
Add olives and finish: About 20 minutes before serving, stir in the Kalamata olives. Taste the sauce and adjust salt, pepper, or lemon as needed.
Serve: Top with crumbled feta and fresh parsley or dill. Spoon over rice, orzo, couscous, roasted potatoes, or tuck into warm pita with a dollop of tzatziki.
Optional thickening: If you want a thicker sauce, remove the chicken and whisk 1 teaspoon cornstarch with 1 tablespoon cold water.
Stir into the liquid, cover, and cook on High for 10 minutes until slightly thickened. Return chicken.